Improving nuclear detection with new chip power

Washington University scientists part of NNSA university-based research collaboration

A cross-disciplinary team of chemists and physicists from Washington University in St. Louis is building a better computer chip to improve detection and surveillance for the illegal transport of nuclear materials at U.S. borders. The work is part of a new, five-year, $10 million collaboration in low-energy nuclear science led by Texas A&M University.

Nuclear & Radiochemistry group
Senior members of the Washington University nuclear program span the chemistry, physics and engineering disciplines, including (from left) Willem Dickhoff, Lee Sobotka, Robert Charity and Jon Elson, along with George Engel (right) of Southern Illinois University Edwardsville (Image: Gary Broyles, Washington University)

Washington University is one of several institutions participating in the Department of Energy/National Nuclear Security Administration’s (DOE/NNSA) Center for Excellence in Nuclear Training and University-based Research (CENTAUR).

Under the new program, Robert J. Charity, research professor of chemistry, and Lee G. Sobotka, professor of chemistry and of physics, both in Arts & Sciences, are testing a novel neutron detection strategy and a related chip. The chip is being developed with long-time collaborator George Engel, a professor in the department of electrical and computer engineering at Southern Illinois University Edwardsville. A kickoff meeting for the CENTAUR collaboration was held Aug. 17.

Related lecture

Chemistry Department Seminar:
“Fun and Games with God’s Quantum Dots”
4 p.m. Thursday, Aug. 30
McMillen Laboratory 311 on the Danforth Campus

Roughly two dozen scientists across all partner universities will be involved in CENTAUR, along with their affiliated research groups. One of the center’s major contributions will be research and development expertise related to neutron detectors, which are relevant for both basic low-energy nuclear science and nuclear security applications.

“The problem with existing neutron detectors is that they are too big to get fine position information,” Sobotka said. “They needed to be big to get the required detection efficiency. The solution is to have many — tens of thousands — of small detectors. This had not been contemplated before as it requires a signal processing stream for each of the small detectors.”

A need for custom processing

ASICs — Application-Specific Integrated Circuits — form the backbone for data processing in computers, cell phones and other electronic devices. These custom chips are made because collecting oft-repeated tasks on one chip makes the overall task faster and less expensive to replicate.

Scientists don’t typically get involved with building their own ASICs, unless there is a highly specific need for the custom processing.

ASIC
Electronic design of an Application-Specific Integrated Circuit (ASIC) developed by scientists at Washington University and SIUE. The collaboration has developed chips specifically for studying the properties of, and reactions between, atomic nuclei. (Image: Nuclear & Radiochemistry group)

For example, ASICs are developed for certain high-energy physics experiments, like those done at the European laboratory near Geneva — CERN — where the Higgs boson was discovered. ASICs are also used in some experiments in space and for medical physics devices like the Positron Emission Tomography (PET) device, which was developed by scientists from Washington University 40 years ago.

For their part, Sobotka, Charity and Jon Elson, research engineer in chemistry, teamed up with Engel to build their own ASICs starting in 2001.

The collaboration has recently upgraded two chips that they built and is making a third one honed for a different scientific task. Using the previous versions of just one of these chip designs, the Washington University group has published 25 papers, mostly on the structure of nuclei with exotic neutron-to-proton ratios (see sidebar).

Not just chips off the old block

Novel ASICs developed by current and former members of the Washington University radiochemistry group have enabled more than 25 scientific papers mostly on the structure of nuclei with exotic neutron-to-proton ratios. These works include:

  • Studying how nuclei can decay by emitting two protons (thesis of Kyle Brown and undergraduate projects of Kevin Mercurio, Marika Jager, Tim Wiser and Walter Buhro);
  • the discovery of exotic isotopes like Na-17 and O-11 (theses of Kyle Brown and Tyler Webb, respectively);
  • how C-12 is made by analyzing how one particular excited state decays (undergraduate project of Juan Manfredi);
  • finding and explaining a way to generate aligned nuclear spins (thesis project of Dan Hoff); and
  • other insights about how some nuclear states seem fortuitously positioned to allow for the synthesis of the elements.

Custom ASICs developed by this group are now used by researchers at Michigan State University, Florida State University, Louisiana State University, Oak Ridge National Laboratory, Texas A&M University and most recently the Japanese lab RIKEN.

CENTAUR researchers will use two of these chips in tandem, coupled with a particular organic crystal as their detector medium, to complete high-resolution experiments with neutrons that current detectors and signal processing electronics do not allow.

“The NNSA will be closely watching this project,” Sobotka said.

Educating the next generation of science leaders

CENTAUR is equally committed to building upon the consortium’s collective tradition of service as a technical resource and fertile training ground for the nation’s nuclear workforce and future stewardship science leaders.

In this vein, the Washington University nuclear groups have a long history of technology development, a bug picked up by their students.

Sobotka highlights the technical contributions of an earlier generation of students, including Edward Hoffman and Michael E. Phelps (former students of  Demetrios Sarantites, professor of chemistry) for their role in the invention of PET and, more recently, James Dempsey (Sobotka’s former student), who invented the ViewRay technology, which allows for real-time clear imaging of tumors as treatment is being delivered.

“Research that advances basic science, like the work supported by CENTAUR, can inspire students to pursue a career of technical innovation that makes a difference in the lives of people across the country — and around the world,” Sobotka said.

Predicting the location of neutrons

The CENTAUR grant will also allow the researchers to improve an advanced model that unifies the quantum structure and reactions of nuclei.

Willem H. Dickhoff, professor of physics in Arts & Sciences, who has worked with Charity for a decade, developed this model to predict the location of neutrons in heavy nuclei.

Nuclear scientists have known the proton distribution for decades, but learning the location of neutrons is a far more difficult task.

Knowing where the neutrons are in large nuclei provides insight into the size of neutron stars. Working with physics graduate students Hossein Mahzoon and Mackenzie Atkinson, Dickhoff and Charity recently published work that indicates that — in one nucleus with more neutrons than protons, Ca-48 — more of the excess neutrons are located further from the center than previously thought.

The CENTAUR grant will allow the researchers to expand the model to other nuclei by gathering more data of the type that Charity, Sobotka and their students including Rebecca Shane, Cole Pruitt and undergraduate Jonathan Mueller have collected over the past decade. Interestingly, some of this work can be completed using the synchrocyclotron at the S. Lee Kling Proton Therapy Center at the Siteman Cancer Center.

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